In addition to comfrey, the number one champion for generating biomass is some kind of grass. Whether annual (like ryegrass) or perennial (fescue), it produces a lot of bulk, has good protein (nitrogen) content. This assumes you have a lawn mower with a bagger! Avoid problematic or weedy grass species, grow what grows well in your area.
Turnips are also a good choice. The seed is fairly cheap, sow them more thickly than you would for a root crop. You can harvest young plants for turnip greens (healthy and tasty). Harvest for compost when they bolt.
Never miss an opportunity to collect fallen brown leaves. From trees, shrubs, anything.